Scientists discover polar Bloch points in strained ferroelectric films

A Bloch point is a singular point around which the field vectors are oriented in nearly all directions. In magnetics, it is the natural link between classical and quantum magnetism, and it has not been directly observed. In ferroelectrics, it has only been predicted in a few cases.

Researchers from the Institute of Metal Research (IMR) of the Chinese Academy of Sciences (CAS) and collaborators from the Institute of Physics of CAS have directly observed polar Bloch points in strained ferroelectric films.

Their work is published in Nature Communications.

Based on their previous work on the polar meron lattice, the researchers considered the model of a tensile-strained ultrathin ferroelectric PbTiO₃ film sandwiched by symmetric electrodes in phase-field simulations and found that the merons transform into Bloch points with the increase of the electrode thickness.

Then, a trilayer SrRuO₃/PbTiO₃/SrRuO₃ film was grown on the SmScO₃ substrate by pulsed laser deposition, and aberration-corrected scanning transmission electron microscopic imaging was used to observe the polarization configuration of polar Bloch points. Further phase-field simulations predicted that a region of negative capacitance exists around each polar Bloch point.

The discovery of polar Bloch points expands the assembly of topological ferroelectric domain structures and implies novel applications in future integrated circuits and low-power electronic devices.